Time-Resolved Soft X-Ray Absorption Spectroscopy of Molecules in the Gas and Liquid Phases

Author:   Cédric Schmidt
Publisher:   Springer Nature Switzerland AG
Edition:   1st ed. 2021
ISBN:  

9783030678401


Pages:   119
Publication Date:   17 February 2022
Format:   Paperback
Availability:   Manufactured on demand   Availability explained
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Time-Resolved Soft X-Ray Absorption Spectroscopy of Molecules in the Gas and Liquid Phases


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Overview

This work studies the relaxation dynamics of molecules in both the gas and liquid phases after strong field ionization, using transient absorption in the soft X-rays. In particular, the thesis presents the first realization of time-resolved X-ray absorption spectroscopy in the spectral water window with a laser-based HHG source. These remarkable experiments were not only performed for isolated molecules, but also in liquids, for which the spectral coverage of the K-edges of C, N, and O are of primary importance for investigating biological molecules. The technique relies on the generation of high-order harmonics to further probe the electronic structure of molecules. Using the atomic selectivity of high energies and the temporal coherence of laser technology, we demonstrate the observation of the first stages of chemical transformation of matter in the gas and liquid phases. 

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Author:   Cédric Schmidt
Publisher:   Springer Nature Switzerland AG
Imprint:   Springer Nature Switzerland AG
Edition:   1st ed. 2021
Weight:   0.221kg
ISBN:  

9783030678401


ISBN 10:   3030678407
Pages:   119
Publication Date:   17 February 2022
Audience:   Professional and scholarly ,  Professional & Vocational
Format:   Paperback
Publisher's Status:   Active
Availability:   Manufactured on demand   Availability explained
We will order this item for you from a manufactured on demand supplier.

Table of Contents

Introduction.- Theoretical Background.- Method and Setup Description.- Time-resolved XAS of Gas Dissociations.- Pulse Peak Power Optimiza@on With Filamentation.

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